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176763

Preparation, Spectral Characterization, DFT and Antibacterial Study of New Azo Ligand Derived From 2-aminoanthracene-9,10-dione With Antipyrine Mixed Ligand Complexes Involving 1,10-phenanthroline Ligand

Article

Last updated: 22 Jan 2023

Subjects

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Tags

Inorganic chemistry

Abstract

Anew azo dye ligand 2-(1,5-dimethyl-3-oxo-2-phenyl-2,3-dihydro-1H-pyrazol-4-yl)diazenyl)anthracene-9,10-dione. was synthesized by the diazotization of 9,10-dioxo-9,10-dihydroanthracene-2-diazonium chloride, and coupling with Antipyrine in alkaline alcoholic solution under suitable optimized experimental conditions to yield a new azo dye (Azo-Anthq-Ap) 2-(diazynyl)anthracene-9,10-dione 4-Antipyrine ligand and react with 1,10-phenanthroline,The structure of mixed-ligand Tetradentate its complexes was prepared from Ni(II), Fe(II) Cu(II) ,Co(II) , Zn(II), and, Hg(II) ions. They confirmed by UV-visb,XRD, (TG, DSC) thermal analysis. FT-IR , 1HMNR spectroscopic methods magnetic susceptibility, elemental analysis, atomic absorption, and molar conductance. The isolated solid complexes are found to have the general formula [M (L)(phen) Cl2] and [M (L)(phen)(H2O)Cl] Cl, conductivity measurements for prepared complexes showed [1:1] electrolyte for Fe(II), and non-electrolyte for the Ni(II), Cu(II),Co(II) Zn(II), and, Hg(II) complexes. The spectral and analytical data revealed that this ligand behaves as a Bidentate chelating agent and coordination number of all metal ions were found to be Six Shape. Finally The synthesized Ligand and metal complexes were screened for their Antibacterial activity against bacterial species, one Gram positive bacteria (Staphylococcus aureus) and three Gram negative bacteria Escherichia coli, Pseudomonas aereuguinosa and Klebsiella pneumoniaea. and, it was found that these compounds show different activity of inhibition on the growth of the bacteria.

DOI

10.21608/ejchem.2021.77118.3774

Keywords

Az 2-aminoanthracene-9, 10-dione, Mixed ligand, 1, 10-phenanthroline

Authors

First Name

Faris Subhi

Last Name

Al alsultan

MiddleName

-

Affiliation

Department of Chemistry/ College of Sciences ,University of Mousel.Iraq .

Email

scp64@student.uomosul.edu.iq

City

-

Orcid

-

First Name

Rana A.S.

Last Name

Al Quaba

MiddleName

-

Affiliation

Department of Chemistry/ College of Sciences ,University of Mousel.Iraq .

Email

-

City

-

Orcid

-

Volume

64

Article Issue

11

Related Issue

27064

Issue Date

2021-11-01

Receive Date

2021-05-22

Publish Date

2021-11-01

Page Start

6,635

Page End

6,646

Print ISSN

0449-2285

Online ISSN

2357-0245

Link

https://ejchem.journals.ekb.eg/article_176763.html

Detail API

https://ejchem.journals.ekb.eg/service?article_code=176763

Order

50

Type

Original Article

Type Code

297

Publication Type

Journal

Publication Title

Egyptian Journal of Chemistry

Publication Link

https://ejchem.journals.ekb.eg/

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Details

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Article

Created At

22 Jan 2023