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69923

Synthesis, Characterization and Microbicides Activities of N-(hydroxy-4-((4-nitrophenyl)diazenyl) benzylidene)-2-(phenylamino)Acetohydrazide Metal Complexes

Article

Last updated: 22 Jan 2023

Subjects

-

Tags

Inorganic chemistry

Abstract

VO(II), Cu(II), Ni(II), Co(II), Mn(II), Fe(III), Ru(III) , Zn(II) and UO2(II) complexes of hydra-zone ligand containing azo group as side chain were prepared from condensation of 2-hydroxy-4-((4-nitrophenyl)diazenyl) benzylidene)benzaldehyde with 2-(phenyl amino)acetohydrazide. The ligand and its complexes were isolated in solid state and characterized by analytical techniques such as elemental analyses, molar conductance, magnetic susceptibility measurements and Electronic spin resonance (ESR) as well as spectroscopic techniques such as UV-Visible, IR, 1H-NMR and 13C- NMR. The spectral data indicated that the ligand acted as neutral bidentate or monobasic tridentate ligand bonded to the metal ions through an oxygen atom of ketonic or enolic carbonyl group, an azomethine nitrogen atom and deprotonated phenolic oxygen atom forming either tetragonally distorted octahedral or square planer geometry. ESR spectra of the solid metal complexes (2-6) and (8) were studied. Antimicrobial activities of the ligand and its complexes were evaluated against E. coli, Bacillus subtilis and Aspergillus Niger by well diffusion method. Results showed that the complex (10) exhibited higher antifungal activity, complex (7) exhibited higher antibacterial than the other complexes against E. coli, while complex (10) exhibited higher antibacterial against B.subtilis than the other complexes.

DOI

10.21608/ejchem.2020.20906.2256

Keywords

Azohydrazone, acetohydrazide, Metal complexes, Bioactivity, ESR

Authors

First Name

Ahmed

Last Name

Alhakimi

MiddleName

Noman

Affiliation

Department of Chemistry, College of Science ,Qassim University, SA

Email

alhakemi10@yahoo.com

City

-

Orcid

‎0000-0002-5141-9333

Volume

63

Article Issue

4

Related Issue

10590

Issue Date

2020-04-01

Receive Date

2019-12-16

Publish Date

2020-04-01

Page Start

1,509

Page End

1,525

Print ISSN

0449-2285

Online ISSN

2357-0245

Link

https://ejchem.journals.ekb.eg/article_69923.html

Detail API

https://ejchem.journals.ekb.eg/service?article_code=69923

Order

25

Type

Original Article

Type Code

297

Publication Type

Journal

Publication Title

Egyptian Journal of Chemistry

Publication Link

https://ejchem.journals.ekb.eg/

MainTitle

-

Details

Type

Article

Created At

22 Jan 2023